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14, 99 (1953). 11. D. Ilkovic, Collect. Czech. Chem. Commun. 6, 498 (1934). 12. S. G. Mairanovskii and M. B. Neiman, Izv. Akad. Nauk SSSR, Otd. Khim. Nauk No. 3, p. 420 (1955). 13. J. J. Lingane and B. A. Loveridge, /. Amer. Chem. Soc. 66, 1425 (1944); 68, 395 (1946); 72, 438(1950). 14. A. Cizek and J. Koutecky, Collect. Czech. Chem. Commun. 28, 2808 (1963). 15. S. G. Mairanovskii, "Catalytic and Kinetic Waves in Polarography" (English translation) Plenum, New York, 1968. 16. C. N. Reilley and W.
The diffusion current for the reverse reaction is therefore expressed in a similar manner. 8) Since the bulk concentration of the product is negligible Eq. 9) and therefore the concentration of the product at the surface is expressed as (Co). 10) Substitution of the expressions for (CR)S and (C 0 ) s in the equation for the reversible electrode potential gives the equation for the i-E wave. B. Irreversible Polarographic Behavior Although many organic electrode processes involve a reversible electrontransfer step, the overall reactions are polarographically irreversible owing to chemical reactions subsequent to the electron transfer.
Academic Press, New York, 1966. 4. P. " Wiley (Interscience), New York, 1954. 5. O. H. Muller, in "Physical Methods of Organic Chemistry" (A. ), Vol. I, Part IV, p. 3155. Wiley (Interscience), New York, 1960. 6. P. " Macmillan, New York, 1964. 7. C. L. Perrin, Prog. Phys. Org. Chem. 3, 165 (1965). 8. P. Zuman and S. Wawzonek, in "Progress in Polarography" (P. Zuman and I. M. ), Vol. I, p. 303. Wiley (Interscience), New York, 1962. 9. J. E. Page, Quart. , Chem. Soc. 6, 262 (1952). 10. P. J. Elving, Ree.